Exploration of pipecolate sulfonamides as binders of the FK506-binding proteins 51 and 52

J Med Chem. 2012 May 10;55(9):4123-31. doi: 10.1021/jm201747c. Epub 2012 Apr 19.

Abstract

FK506-binding proteins (FKBP) 51 and 52 are cochaperones that modulate the signal transduction of steroid hormone receptors. Single nucleotide polymorphisms in the gene encoding FKBP51 have been associated with a variety of psychiatric disorders. Rapamycin and FK506 are two macrocyclic natural products, which tightly bind to most FKBP family members, including FKBP51 and FKBP52. A bioisosteric replacement of the α-ketoamide moiety of rapamycin and FK506 with a sulfonamide was envisaged with the retention of the conserved hydrogen bonds. A focused solid support-based synthesis protocol was developed, which led to ligands with submicromolar affinity for FKBP51 and FKBP52. The molecular binding mode for one sulfonamide analogue was confirmed by X-ray crystallography.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Crystallography, X-Ray
  • Fluorescence Polarization
  • Humans
  • Magnetic Resonance Spectroscopy
  • Molecular Structure
  • Pipecolic Acids / chemical synthesis*
  • Pipecolic Acids / chemistry
  • Pipecolic Acids / pharmacology
  • Protein Binding
  • Spectrometry, Mass, Electrospray Ionization
  • Structure-Activity Relationship
  • Sulfonamides / chemical synthesis*
  • Sulfonamides / chemistry
  • Sulfonamides / pharmacology
  • Tacrolimus / analogs & derivatives*
  • Tacrolimus / chemical synthesis
  • Tacrolimus / chemistry
  • Tacrolimus / pharmacology
  • Tacrolimus Binding Proteins / antagonists & inhibitors
  • Tacrolimus Binding Proteins / metabolism*

Substances

  • Pipecolic Acids
  • Sulfonamides
  • Tacrolimus Binding Proteins
  • tacrolimus binding protein 4
  • tacrolimus binding protein 5
  • Tacrolimus